Structure and Mesophases of Hexacyclen Derivatives

Reference:

S. H. J. Idziak, N. C. Maliszewskyj, P. A. Heiney, J. P. McCauley, Jr., P. A. Sprengler, and A. B. Smith, III, J. Am. Chem. Soc. 113, 7666-7672 (1991).

Abstract:

A variety of hexacyclene derivatives with aliphatic substituents have been prepared and characterized via X-ray diffraction, calorimetry, thermogravimetric analysis, and computer simulations. A subset of these compounds are seen to display a liquid crystalline mesophase, while others transform directly from the crystalline to the isotropic liquid phase. The merits of tubular and smectic liquid crystalline models for the mesophase structure are discussed.


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